Determination of free d-alanine in the human plasma by capillary electrophoresis with optical fiber light-emitting diode-induced fluorescence detection [An article from: Analytica Chimica Acta]

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Description:
A new analytical method for d-alanine (d-Ala) based on capillary electrophoretic separation and optical fiber light-emitting diode (LED)-induced fluorescence detection has been developed. Fluorescein isothiocyanate (FITC) was used for precolumn derivatization of amino acids. The separation and determination of the derivatives was performed using a novel laboratory-built CE system with optical fiber LED-induced fluorescence detector. Optimal separation was performed at 15kV using a background electrolyte solution consisted of 25mmolL^-^1 sodium borate (pH 9.5), 18mmolL^-^1 @b-CD and 15mmolL^-^1 SDS. High sensitive detection was obtained by the optical fiber LED-induced fluorescence detection using a blue LED as the excitation source. The limits of detection (S/N=3) for d-Ala was 8.0×10^-^9molL^-^1. A calibration curve ranging from 2.0×10^-^8molL^-^1 to 1.0×10^-^6molL^-^1 was shown to be linear. Using this method, the levels of d-Ala in human plasma from healthy donors were determined.

Determination of free d-alanine in the human plasma by capillary electrophoresis with optical fiber light-emitting diode-induced fluorescence detection [An article from: Analytica Chimica Acta]

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